Dasgupta, Chandan and Valls, Oriol T (1998) Entropic origin of the growth of relaxation times in simple glassy liquids. In: Physical Review, 58 (01). pp. 801-804.
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Abstract
Transitions between "glassy" local minima of a model free-energy functional for a dense hard-sphere system are studied numerically using a "microcanonical" Monte Carlo method that enables us to obtain the transition probability as a function of the free energy and the Monte Carlo "time." The growth of the height of the effective free-energy barrier with density is found to be consistent with a Vogel-Fulcher law. The dependence of the transition probability on time indicates that this growth is primarily due to an increase in the difficulty of finding low-free-energy paths to other minima.
Item Type: | Journal Article |
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Publication: | Physical Review |
Publisher: | American Physical Society |
Additional Information: | Copyright of this article belongs to American Physical Society. |
Department/Centre: | Division of Physical & Mathematical Sciences > Physics |
Date Deposited: | 15 Jul 2009 10:14 |
Last Modified: | 19 Sep 2010 05:24 |
URI: | http://eprints.iisc.ac.in/id/eprint/18568 |
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