Chouhan, Arun Singh and Jasti, Naga Prathibha and Hadke, Shreyash and Raghavan, Srinivasan and Avasthi, Sushobhan (2017) Large grained and high charge carrier lifetime CH3NH3PbI3 thin-films: implications for perovskite solar cells. In: CURRENT APPLIED PHYSICS, 17 (10). pp. 1335-1340.
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Abstract
Spin coated perovslcite thin films are known to have an issue of pinholes & poor morphology control which lead to poor device-to-device repeatability, that is an impediment to scale-up. In this work, Methylamine vapor annealing process is demonstrated which consistently leads to high-quality perovskite thin-films with an average grain-size of 10-15 mu m. The improvement in film morphology enables improvement in effective carrier recombination lifetime, from 21 its in as-deposited films to 54 mu s in vapor-annealed films. The annealed films with large-grains are also more stable in ambient conditions. Devices made on annealed perovskite films are very consistent, with a standard deviation of only 0.7%. Methylamine vapor annealing process is a promising method of depositing large-grain CH3NH3PbI3 films with high recombination lifetime and the devices with improved performance. (C) 2017 Elsevier B.V. All rights reserved.
Item Type: | Journal Article |
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Publication: | CURRENT APPLIED PHYSICS |
Additional Information: | Copy right for this article belongs to the ELSEVIER SCIENCE BV, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS |
Department/Centre: | Division of Interdisciplinary Sciences > Centre for Nano Science and Engineering |
Date Deposited: | 23 Sep 2017 05:11 |
Last Modified: | 23 Sep 2017 05:11 |
URI: | http://eprints.iisc.ac.in/id/eprint/57853 |
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