Investigations of aerosol black carbon from a semi-urban site in the Indo-Gangetic Plain region

Joshi, Hema and Naja, Manish and Singh, KP and Kumar, Rajesh and Bhardwaj, P and Babu, Suresh S and Satheesh, SK and Moorthy, Krishna K and Chandola, HC (2016) Investigations of aerosol black carbon from a semi-urban site in the Indo-Gangetic Plain region. In: ATMOSPHERIC ENVIRONMENT, 125 (B, SI). pp. 346-359.

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Abstract

Long-term (2009-2012) data from ground-based measurements of aerosol black carbon (BC) from a semi-urban site, Pantnagar (29.0 degrees N, 79.5 degrees E, 231 m amsl), in the Indo-Gangetic Plain (IGP) near the Himalayan foothills are analyzed to study the regional characterization. Large variations are seen in BC at both diurnal and seasonal scales, associated with the mesoscale and synoptic meteorological processes, and local/regional anthropogenic activities. BC diurnal variations show two peaks (morning and evening) arising from the combined effects of the atmospheric boundary layer (ABL) dynamics and local emissions. The diurnal amplitudes as well as the rates of diurnal evolution are the highest in winter season, followed by autumn, and the lowest in summer-monsoon. BC exhibits nearly an inverse relation with mixing layer depth in all seasons; being strongest in winter (R-2 = 0.89) and weakest (R-2 = 0.33) in monsoon (July-August). Unlike BC, co-located aerosol optical depths (AOD) and aerosol absorption are highest in spring over IGP, probably due to the presence of higher abundances of aerosols (including dust) above the ABL (in the free troposphere). AOD (500 nm) showed annual peak (>0.6) in May-June, dominated by coarse mode, while fine mode aerosols dominated in late autumn and early winter. Aerosols profiles from CALIPSO show highest values close to the surface in winter/autumn, similar to the feature seen in surface BC, whereas at altitudes > 2 km, the extinction is maximum in spring/summer. WRF-Chem model is used to simulate BC temporal variations and then compared with observed BC. The model captures most of the important features of the diurnal and seasonal variations but significantly underestimated the observed BC levels, suggesting improvements in diurnal and seasonal varying BC emissions apart from the boundary layer processes. (C) 2015 Elsevier Ltd. All rights reserved.

Item Type:	Journal Article
Publication:	ATMOSPHERIC ENVIRONMENT
Publisher:	PERGAMON-ELSEVIER SCIENCE LTD
Additional Information:	Copy right for this article belongs to the PERGAMON-ELSEVIER SCIENCE LTD, THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
Keywords:	Aerosols; Black carbon; Aerosol optical depth; Boundary layer; Indo-Gangetic Plain; Himalayas
Department/Centre:	Division of Mechanical Sciences > Centre for Atmospheric & Oceanic Sciences
Date Deposited:	10 Feb 2016 05:52
Last Modified:	10 Feb 2016 05:52
URI:	http://eprints.iisc.ac.in/id/eprint/53197

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